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(Similar effects are anticipated for basic monomers) Several mechanisms have been proposed to describe the results for nonionizable monomers: radical solvent complexation, monomer solvent complexation, and the bootstrap effect Complexation of the polar solvent with the more polar monomer or radical decreases the reactivity of the more polar monomer or radical The bootstrap effect results from partitioning of the two monomers between the solution and the local feed composition in the domain of the growing polymer radical Copolymers are richer in the less polar monomer for reaction in polar solvents because the local feed composition is richer in the less polar monomer The magnitude of the bootstrap effect can be signi cant depending on the difference in polarity of the two monomers [Coote et al, 1998].

[1] Blaunstein, N., and J. Bach Andersen, Multipath Phenomena in Cellular Networks, Artech House Boston-London, 2002. [2] Blaunstein, N., and Y. Ben-Shimol, Spectral properties of signal fading and Doppler spectra distribution in urban mobile communication links, Wireless Communic. and Mobile Computing, vol. 5, no. 1, 2006, pp. 113 116. [3] Ponomarev, G. A., A. N. Kulikov, and E. D. Telpukhovsky, Propogation of Ultra Short Waves in Urban Environments, Tomsk, Rasko, USSR, 1991. [4] Pedersen, K., P. E. Mogensen, and B. Fleury, Power azimuth spectrum in outdoor environments, IEE Electron. Letters, vol. 33., 1997, pp. 1583 1584. [5] Pedersen, K. I., B. H. Fleury, and P. E. Mogensen, High resolution of electromagnetic waves in time-varying radio channels, IEEE Proc. Personal, Indoor, and Mobile Radio Communic. (PIMRC 97), Helsinki, Finland, Sept. 1997, pp. 650 654. [6] Pedersen, K. I., P. Mogensen, and B. H. Fleury, Experimental analysis of the joint statistical properties of azimuth spread, delay spread, and shadow fading, IEEE J. Select. Areas Communic., vol. 20, no. 3, 2002 pp. 523 531.

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Thus, for 2-hydroxyethylmethacrylate (M1)-t-butyl acrylate (M2), r1 4:35 and r2 0:355 in bulk copolymerization compared to r1 1:79 and r2 0:510 in copolymerization in DMF [Fernandez Monreal et al, 2001] For a comonomer pair with a smaller difference in polarity such as styrene (M1)-n-butyl acrylate (M2), r1 0:865 and r2 0:189 in bulk compared to r1 0:734 and r2 0:330 [Fernandez Garcia et al, 2000] 6-3a-2 Temperature.

An examination of various compilations of monomer reactivity ratios [Greenley, 1989a, 1999; Young, 1975] shows that r1 and r2 are relatively insensitive to temperature provided that propagation is irreversible. Thus the r1 and r2 values for styrene-1,3-butadiene are 0.64 and 1.4 at 5 C, and 0.60 and 1.8 at 45 C. The r1 and r2 values for styrene methyl methacrylate are 0.52 and 0.46 at 60 C, and 0.59 and 0.54 at 131 C. The monomer reactivity ratio is the ratio of two propagation rate constants, and its variation with temperature will depend on the difference in propagation activation energies according to

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[7] Pedersen, K, P Mogensen, and B Fleury, A stochastic model of the temporal and azimuthal dispersion seen at the base station in outdoor propagation environments, IEEE Trans Veh Technol, vol 49, no 2, 2000, pp 437 447 [8] Ertel, R B, P Cardieri, K W Sowerby et al Overview of spatial channel models for antenna array communications systems, IEEE Personal Communic, vol 5, no 1, 1998, pp 10 22 [9] Fuhl, J, J P Rossi, and E Bonek, High resolution 3-D direction-of-arrival determination for urban mobile radio, IEEE Trans Antennas Propagat, vol 44, no 4, 1997, pp 672 682 [10] Kuchar, A, J P Rossi, and E Bonek, Directional macro-cell channel characterization from urban measurements, IEEE Trans Antennas Propagat, vol 48, no 1, 2000, pp 137 146 [11] Kalliola, K, H Laitenen, L Vaskelainen et al.

r1 ! k11 A11 E12 E11 exp RT k12 A12 6-48

, Real-time 3-D spatial-temporal dualpolarized measurement of wideband radio channel at mobile station, IEEE Trans Instrum Measurements, vol 49, no 3, 2000, pp 439 448 [12] Kalliola, K, and P Vainikainen, Characterization system for radio channel of adaptive array antennas, Proc Int Symp Personal Indoor Mobile Radio Conf (PIRMC 97), Helsinki, Finland, 1997, pp 95 99 [13] Laurila, J, K Kalliola, M Toeltsch et al, Wide-band 3-D characterization of mobile radio channels in urban environment, IEEE Trans Antennas Propagat, vol 50, no 2, 2002, pp 233 243 [14] Toeltsch, M, J Laurila, K Kalliola et al, Statistical characterization of urban spatial radio channels, IEEE J Select Areas Communic, vol 20, no 3, 2002, pp 539 549 [15] Blaunstein, N, M Toeltsch, E Benek et al.

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